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Perspective—Multinary Oxide Semiconductors for Solar Fuels Generation: Closing the Performance Gap between Theory and Practice

https://doi.org/10.1149/2162-8777/ac689c

O’Donnell, Shaun ; Vali, Abbas ; Rawat, Abhishek ; Maggard, Paul A. ; Huda, Muhammad N. ; Rajeshwar, Krishnan ( May 2022 , ECS Journal of Solid State Science and Technology)

This Perspective addresses the current state-of-the-art with the development of multinary oxides—a family of compounds that has long interested Prof. John B. Goodenough. Specifically, here we focus on their use as photoelectrodes for solar fuels generation. Using optical data and assuming an idealized 100% incident photon-to-electron conversion efficiency, it is possible to project the maximum short circuit photocurrent efficiency to be expected for a given oxide semiconductor. The performance gap between this theoretical value and that realized experimentally, is shown to be sizable for all but a couple of candidates. The technical issues underlying this gap and strategies for closing it are presented below.
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Role of f -electrons in determining insulator to metal phase transitions of Ca(La 1−x Ce x ) 2 S 4 (0 ≤ x ≤ 1) solid solution: A DFT + U study

https://doi.org/10.1063/5.0058096

Sarker, Hori Pada ; Huda, Muhammad N. ( October 2021 , Journal of Applied Physics)
First-principles study on the effect of Sn doping in Cu 2 S—Acanthite phase as a substitute to low chalcocite for modeling complex doping

https://doi.org/10.1063/5.0008499

Barman, Sajib K. ; Huda, Muhammad N. ( July 2020 , Journal of Applied Physics)
Niobium Doping in BiVO 4 : Interplay Between Effective Mass, Stability, and Pressure

https://doi.org/10.1002/cphc.201800792

Sarker, Hori Pada ; Rao, Pratap M. ; Huda, Muhammad N. ( February 2019 , ChemPhysChem)
Electrodeposition of Silver Vanadate Films: A Tale of Two Polymorphs

https://doi.org/10.1002/cphc.201900558

Vali, Abbas ; Sarker, Hori P. ; Jee, Hyung‐Woo ; Kormányos, Attila ; Firouzan, Farinaz ; Myung, Noseung ; Paeng, Ki‐Jung ; Huda, Muhammad N. ; Janáky, Csaba ; Rajeshwar, Krishnan ( September 2019 , ChemPhysChem)